TY - JOUR
T1 - Rise of Metal-Organic Frameworks
T2 - From Synthesis to E-Skin and Artificial Intelligence
AU - Sun, Qi Jun
AU - Guo, Wen Tao
AU - Liu, Shu Zheng
AU - Tang, Xin Gui
AU - Roy, Vellaisamy AL
AU - Zhao, Xin Hua
N1 - Publisher Copyright:
© 2024 American Chemical Society
PY - 2024/9/4
Y1 - 2024/9/4
N2 - Metal-organic frameworks (MOFs) have attained broad research attention in the areas of sensors, resistive memories, and optoelectronic synapses on the merits of their intriguing physical and chemical properties. In this review, recent progress on the synthesis of MOFs and their electronic applications is introduced and discussed. Initially, the crystal structures and properties of MOFs encompassing optical, electrical, and chemical properties are discussed in brief. Subsequently, advanced synthesis methods for MOFs are introduced, categorized into hydrothermal approach, microwave synthesis, mechanochemical synthesis, and electrochemical deposition. After that, the various roles of MOFs in widespread applications, including sensing, information storage, optoelectronic synapses, machine learning, and artificial intelligence, are discussed, highlighting their versatility and the innovative solutions they provide to long-standing challenges. Finally, an outlook on remaining challenges and a future perspective for MOFs are proposed.
AB - Metal-organic frameworks (MOFs) have attained broad research attention in the areas of sensors, resistive memories, and optoelectronic synapses on the merits of their intriguing physical and chemical properties. In this review, recent progress on the synthesis of MOFs and their electronic applications is introduced and discussed. Initially, the crystal structures and properties of MOFs encompassing optical, electrical, and chemical properties are discussed in brief. Subsequently, advanced synthesis methods for MOFs are introduced, categorized into hydrothermal approach, microwave synthesis, mechanochemical synthesis, and electrochemical deposition. After that, the various roles of MOFs in widespread applications, including sensing, information storage, optoelectronic synapses, machine learning, and artificial intelligence, are discussed, highlighting their versatility and the innovative solutions they provide to long-standing challenges. Finally, an outlook on remaining challenges and a future perspective for MOFs are proposed.
KW - Artificial intelligence
KW - E-skin
KW - Information storage
KW - Metal−organic frameworks
KW - Optoelectronic synapse
UR - http://www.scopus.com/inward/record.url?scp=85201910263&partnerID=8YFLogxK
U2 - 10.1021/acsami.4c07732
DO - 10.1021/acsami.4c07732
M3 - Review article
C2 - 39178336
AN - SCOPUS:85201910263
SN - 1944-8244
VL - 16
SP - 45830
EP - 45860
JO - ACS Applied Materials and Interfaces
JF - ACS Applied Materials and Interfaces
IS - 35
ER -