Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Gui Chen; Lingjing Chen; Siu Mui Ng; Wai Lun Man; Tai Chu Lau

doi:10.1002/anie.201209116

Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Gui Chen, Lingjing Chen, Siu Mui Ng, Wai Lun Man, Tai Chu Lau

Research output: Contribution to journal › Article › peer-review

166 Citations (Scopus)

Abstract

Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe ₂O₃ nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000.

Original language	English
Pages (from-to)	1789-1791
Number of pages	3
Journal	Angewandte Chemie - International Edition
Volume	52
Issue number	6
DOIs	https://doi.org/10.1002/anie.201209116
Publication status	Published - 4 Feb 2013
Externally published	Yes

Keywords

iron complexes
iron oxides
solar energy conversion
water oxidation

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10.1002/anie.201209116

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abstract = "Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000.",

keywords = "iron complexes, iron oxides, solar energy conversion, water oxidation",

author = "Gui Chen and Lingjing Chen and Ng, {Siu Mui} and Man, {Wai Lun} and Lau, {Tai Chu}",

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T2 - Evidence for Dual-active intermediates in iron-catalyzed water oxidation

AU - Chen, Gui

AU - Chen, Lingjing

AU - Ng, Siu Mui

AU - Man, Wai Lun

AU - Lau, Tai Chu

PY - 2013/2/4

Y1 - 2013/2/4

N2 - Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000.

AB - Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000.

KW - iron complexes

KW - iron oxides

KW - solar energy conversion

KW - water oxidation

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U2 - 10.1002/anie.201209116

DO - 10.1002/anie.201209116

M3 - Article

AN - SCOPUS:84873375231

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VL - 52

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JO - Angewandte Chemie - International Edition

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Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Abstract

Keywords

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